June Foray

(voice)

Paul Winchell

Gargamel (voice)

Lucille Bliss

Smurfette (voice)

Amanda McBroom

Chlorhydris (voice)

Don Messick

Papa Smurf / Azrael (voice)

Joe Besser

Cupid (voice)

William Callaway

(voice)

Michael Bell

(voice)

Hamilton Camp

(voice)

Danny Goldman

(voice)